I believe that only the melody of a tune can be copyrighted. Chord progressions cannot. If you have permission to use the melody, you can put whatever you want underneath it.
The intention of the performance factors in as well. For-profit concertizing would be viewed more sternly.
PERFORMANCE IN CHURCH is copyright-restriction free. You can sing or play anything you want, any way you want, as much as you want without asking anyone permission or paying for anything at all.
When in Doubt, Do Without
I did a re-harmonization a couple of years ago to a very infamous mass setting. I was given permission to do both, compose a new harmony and print it for the choir. I have not been to confession yet on this one, and unfortunately, it still exists.
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